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Regulating Intrinsic Electronic Structures of Transition-Metal-Based Catalysts and the Potential Applications for Electrocatalytic Water Splitting
Yuan, Cheng Zong1; Hui, Kwan San2; Yin, Hong11; Zhu, Siqi10; Zhang, Jintao3; Wu, Xi Lin4; Hong, Xiaoting5; Zhou, Wei6; Fan, Xi7; Bin, Feng8; Chen, Fuming9; Hui, Kwun Nam1
2021-06-07
Source PublicationACS Materials Letters
Volume3Issue:6Pages:752-780
AbstractEfficient and low-cost transition-metal (TM)-based electrocatalysts have been of great importance for producing hydrogen (H2) and oxygen (O2) via electrocatalytic water (H2O) splitting to ameliorate global energy and environmental problems. However, TM-based materials generally suffer from unsatisfactory electrocatalytic activity because of their relatively low conductivity and unregulated electronic structure. Therefore, the electronic structure engineering of electrocatalysts is an efficient strategic approach to enhance catalytic performances and stabilities. In this review, recent experimental and theoretical advances in the intrinsic electronic structure regulation of TM-based nanomaterials are summarized in terms of preparation methods and underlying natures to boost hydrogen evolution reaction and oxygen evolution reaction. A systematic discussion is conducted on engineering strategies for TM-based nanomaterials to regulate their electronic structures, optimize their adsorption ability of reaction intermediates, and reduce reaction barrier. The existing challenges and perspectives of TM-based electrocatalysts are highlighted to provide new insights into technological advancement for hydrogen production.
DOI10.1021/acsmaterialslett.0c00549
URLView the original
Language英語English
Scopus ID2-s2.0-85106514239
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Cited Times [WOS]:2   [WOS Record]     [Related Records in WOS]
Document TypeJournal article
CollectionUniversity of Macau
Affiliation1.Joint Key Laboratory of the Ministry of Education, Institute of Applied Physics and Materials Engineering, University of Macau, Avenida da Universidade, Taipa, 999078, Macao
2.School of Engineering, Faculty of Science, University of East Anglia, Norwich, NR4 7TJ, United Kingdom
3.School of Chemistry and Chemical Engineering, Shandong University, Jinan, 250061, China
4.College of Geography and Environmental Science, Zhejiang Normal University, Jinhua, 321004, China
5.Department of Chemistry, Zhejiang Sci-tech University, Hangzhou, 310018, China
6.Department of Mechanical and Electrical Engineering, Xiamen University, Xiamen, 361005, China
7.Ningbo Institute of Materials Technology, Engineering, Chinese Academy of Sciences, Ningbo, 315201, China
8.State Key Laboratory of High-Temperature Gas Dynamics, Institute of Mechanics, Chinese Academy of Science, Beijing, 100190, China
9.State Key Laboratory of Optic Information Physics and Technologies, School of Physics and Telecommunication Engineering, South China Normal University, Guangzhou, 510006, China
10.Anhui University of Technology, Huashan District Ma'anshan Anhui, China
11.Applied Materials, Huazhong University of Science and Technology, Hubei, 430074, China
First Author AffilicationINSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING
Recommended Citation
GB/T 7714
Yuan, Cheng Zong,Hui, Kwan San,Yin, Hong,et al. Regulating Intrinsic Electronic Structures of Transition-Metal-Based Catalysts and the Potential Applications for Electrocatalytic Water Splitting[J]. ACS Materials Letters,2021,3(6):752-780.
APA Yuan, Cheng Zong,Hui, Kwan San,Yin, Hong,Zhu, Siqi,Zhang, Jintao,Wu, Xi Lin,Hong, Xiaoting,Zhou, Wei,Fan, Xi,Bin, Feng,Chen, Fuming,&Hui, Kwun Nam.(2021).Regulating Intrinsic Electronic Structures of Transition-Metal-Based Catalysts and the Potential Applications for Electrocatalytic Water Splitting.ACS Materials Letters,3(6),752-780.
MLA Yuan, Cheng Zong,et al."Regulating Intrinsic Electronic Structures of Transition-Metal-Based Catalysts and the Potential Applications for Electrocatalytic Water Splitting".ACS Materials Letters 3.6(2021):752-780.
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