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Commercialization-Driven Electrodes Design for Lithium Batteries: Basic Guidance, Opportunities, and Perspectives
Cao, Chunyan1,2; Liang, Fanghua1; Zhang, Wei1; Liu, Hongchao1,3; Liu, Hui3; Zhang, Haifeng1; Mao, Jiajun4; Zhang, Yanyan4; Feng, Yu5; Yao, Xi2; Ge, Mingzheng1,3; Tang, Yuxin4
Source PublicationSmall

Current lithium-ion battery technology is approaching the theoretical energy density limitation, which is challenged by the increasing requirements of ever-growing energy storage market of electric vehicles, hybrid electric vehicles, and portable electronic devices. Although great progresses are made on tailoring the electrode materials from methodology to mechanism to meet the practical demands, sluggish mass transport, and charge transfer dynamics are the main bottlenecks when increasing the areal/volumetric loading multiple times to commercial level. Thus, this review presents the state-of-the-art developments on rational design of the commercialization-driven electrodes for lithium batteries. First, the basic guidance and challenges (such as electrode mechanical instability, sluggish charge diffusion, deteriorated performance, and safety concerns) on constructing the industry-required high mass loading electrodes toward commercialization are discussed. Second, the corresponding design strategies on cathode/anode electrode materials with high mass loading are proposed to overcome these challenges without compromising energy density and cycling durability, including electrode architecture, integrated configuration, interface engineering, mechanical compression, and Li metal protection. Finally, the future trends and perspectives on commercialization-driven electrodes are offered. These design principles and potential strategies are also promising to be applied in other energy storage and conversion systems, such as supercapacitors, and other metal-ion batteries.

KeywordHigh Energy Density High Mass Loading Lithium Batteries Rational Structure Design Sluggish Charge Diffusion
URLView the original
Indexed BySCIE
WOS Research AreaChemistry ; Materials Science ; Science & Technology - Other Topics ; Physics
WOS SubjectChemistry, Multidisciplinary ; Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary ; Physics, Applied ; Physics, Condensed Matter
WOS IDWOS:000681253900001
Scopus ID2-s2.0-85111722371
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Cited Times [WOS]:1   [WOS Record]     [Related Records in WOS]
Document TypeJournal article
CollectionUniversity of Macau
Corresponding AuthorLiu, Hongchao; Ge, Mingzheng; Tang, Yuxin
Affiliation1.School of Textile and Clothing, Nantong University, Nantong, 226019, China
2.Department of Biomedical Sciences, City University of Hong Kong, 999077, Hong Kong
3.Institute of Applied Physics and Materials Engineering, University of Macau, 999078, Macao
4.College of Chemical Engineering, Fuzhou University, Fuzhou, 350116, China
5.State Key Laboratory of Clean and Efficient Coal Utilization, Key Laboratory of Coal Science and Technology, Ministry of Education, Taiyuan University of Technology, Taiyuan, 030024, China
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GB/T 7714
Cao, Chunyan,Liang, Fanghua,Zhang, Wei,et al. Commercialization-Driven Electrodes Design for Lithium Batteries: Basic Guidance, Opportunities, and Perspectives[J]. Small,2021,17(43).
APA Cao, Chunyan,Liang, Fanghua,Zhang, Wei,Liu, Hongchao,Liu, Hui,Zhang, Haifeng,Mao, Jiajun,Zhang, Yanyan,Feng, Yu,Yao, Xi,Ge, Mingzheng,&Tang, Yuxin.(2021).Commercialization-Driven Electrodes Design for Lithium Batteries: Basic Guidance, Opportunities, and Perspectives.Small,17(43).
MLA Cao, Chunyan,et al."Commercialization-Driven Electrodes Design for Lithium Batteries: Basic Guidance, Opportunities, and Perspectives".Small 17.43(2021).
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