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Microwave-assisted hydrothermal assembly of 2D copper-porphyrin metal-organic frameworks for the removal of dyes and antibiotics from water
Zhao,Shiyin1,2; Li,Shun1,3,4; Zhao,Zhicheng1; Su,Yiping1; Long,Yangke1; Zheng,Zuquan1; Cui,Daling4; Liu,Yong4; Wang,Chunfei2; Zhang,Xuanjun2; Zhang,Zuotai1
2020-11-01
Source PublicationEnvironmental Science and Pollution Research
ISSN0944-1344
Volume27Issue:31Pages:39186-39197
Abstract

Adsorption and photocatalysis are promising strategies to remove pollutants of dyes and antibiotics from wastewater. In this study, we demonstrate a rapid microwave-assisted hydrothermal route for the assembly of 2D copper-porphyrin Metal-Organic Frameworks (Cu-TCPP MOFs) within 1 h. The resulting 2D Cu-TCPP nanosheets with excellent crystallinity and a large surface area (342.72 m/g) exhibited outstanding adsorption performance for typical dyes with adsorption capacities of about 185 mg/g for rhodamine B, 625 mg/g for methylene blue, and 290 mg/g for Congo red, respectively, as well as for representative antibiotics with adsorption capacities of about 130 mg/g for oxytocin, 150 mg/g for tetracycline, and 50 mg/g for norfloxacin, respectively. Meanwhile, the as-prepared 2D Cu-TCPP showed good photocatalytic degradation activity of pollutants after adsorption under irradiation by visible light, reaching removal efficiencies of 81.2 and 86.3% toward rhodamine B and norfloxacin, respectively. These results demonstrate the promising potential of 2D Cu-TCPP for use in the removal of contaminants from wastewater.

KeywordAdsorption Antibiotics Microwave Synthesis Photocatalysis Two-dimensional Mofs
DOI10.1007/s11356-020-09865-z
URLView the original
Indexed BySCIE
Language英語English
WOS Research AreaEnvironmental Sciences & Ecology
WOS SubjectEnvironmental Sciences
WOS IDWOS:000546205500003
Scopus ID2-s2.0-85087631152
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Cited Times [WOS]:12   [WOS Record]     [Related Records in WOS]
Document TypeJournal article
CollectionFaculty of Health Sciences
Biological Imaging and Stem Cell
Corresponding AuthorLi,Shun; Zhang,Xuanjun; Zhang,Zuotai
Affiliation1.School of Environmental Science and Engineering,Guangdong Provincial Key Laboratory of Soil and Groundwater Pollution Control,Southern University of Science and Technology (SUSTech),Shenzhen,518055,China
2.Bioimaging Core,Faculty of Health Sciences,University of Macau,Macao
3.Academy for Advanced Interdisciplinary Studies,Southern University of Science and Technology (SUSTech),Shenzhen,518055,China
4.Foshan (Southern China) Institute for New Materials,Foshan,528200,China
First Author AffilicationFaculty of Health Sciences
Corresponding Author AffilicationFaculty of Health Sciences
Recommended Citation
GB/T 7714
Zhao,Shiyin,Li,Shun,Zhao,Zhicheng,et al. Microwave-assisted hydrothermal assembly of 2D copper-porphyrin metal-organic frameworks for the removal of dyes and antibiotics from water[J]. Environmental Science and Pollution Research,2020,27(31):39186-39197.
APA Zhao,Shiyin,Li,Shun,Zhao,Zhicheng,Su,Yiping,Long,Yangke,Zheng,Zuquan,Cui,Daling,Liu,Yong,Wang,Chunfei,Zhang,Xuanjun,&Zhang,Zuotai.(2020).Microwave-assisted hydrothermal assembly of 2D copper-porphyrin metal-organic frameworks for the removal of dyes and antibiotics from water.Environmental Science and Pollution Research,27(31),39186-39197.
MLA Zhao,Shiyin,et al."Microwave-assisted hydrothermal assembly of 2D copper-porphyrin metal-organic frameworks for the removal of dyes and antibiotics from water".Environmental Science and Pollution Research 27.31(2020):39186-39197.
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