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Synthetic Study toward the Total Synthesis of Taxezopidines A and B
Hu, Ya-Jian; Fan, Jian-Hong; Li, Shaoping; Zhao, Jing; Li, Chuang-Chuang
2018-09-21
Source PublicationORGANIC LETTERS
ISSN1523-7060
Volume20Issue:18Pages:5905-5909
AbstractA concise synthetic approach to construct the [6,8,6]-tricyclic core of taxezopidines A and B, which contains a synthetically challenging bridged bicyclo[5.3.1]undecane ring system bearing most of the desired functionalized groups and stereocenters, has been established. This approach features a diastereoselective type II intramolecular Diels-Alder furan reaction. The stereochemistry of the acetoxy group at the allylic position of the dienophile alkene group, such as in 6a, was found to be critical for achieving the desired highly diastereoselective outcome.
DOI10.1021/acs.orglett.8b02571
URLView the original
Indexed BySCI
Language英语
WOS Research AreaChemistry
WOS SubjectChemistry, Organic
WOS IDWOS:000445711500084
PublisherAMER CHEMICAL SOC
The Source to ArticleWOS
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Document TypeJournal article
CollectionUniversity of Macau
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GB/T 7714
Hu, Ya-Jian,Fan, Jian-Hong,Li, Shaoping,et al. Synthetic Study toward the Total Synthesis of Taxezopidines A and B[J]. ORGANIC LETTERS,2018,20(18):5905-5909.
APA Hu, Ya-Jian,Fan, Jian-Hong,Li, Shaoping,Zhao, Jing,&Li, Chuang-Chuang.(2018).Synthetic Study toward the Total Synthesis of Taxezopidines A and B.ORGANIC LETTERS,20(18),5905-5909.
MLA Hu, Ya-Jian,et al."Synthetic Study toward the Total Synthesis of Taxezopidines A and B".ORGANIC LETTERS 20.18(2018):5905-5909.
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